Theoretical and experimental study of electronic temperatures in heavy ion tracks from Auger electron spectra and thermal spike calculations
نویسندگان
چکیده
Electron spectra were measured at GANIL with different heavy ions (C–Mo) and various charge states q (q = 6–39) at fixed projectile velocity v (v = 19 atomic units, 9.2 MeV/u). A projectile dependent broadening of ion induced KVV Auger electron peaks from carbon targets was observed. From this broadening, one can deduce a mean ‘‘electronic temperature’’ of the heavy ion induced track at the corresponding Auger decay time (10 fs). We compare the measured temperature values to the predictions of an inelastic-thermal spike model, which takes into account the electron–phonon coupling. The model underestimates the experimental values, but reproduces the increase with ion charge. 2005 Elsevier B.V. All rights reserved. PACS: 79.20.Rf; 34.50.Dy; 61.80.Jh
منابع مشابه
Electronic energy-density effects in ion tracks of metals
High resolution Auger-electron spectroscopy has been applied to the interaction of swift heavy ions with atomically clean metallic solids. Spectra have been taken for fast projectile electrons and for charge-state equilibrated ions at normal incidence on micro crystalline beryllium samples, Al(100) single crystals and several metallic glasses (Al87La7Ni5Zr1, Ni78B14Si8, Co66Si16B12Fe4Mo2). From...
متن کاملTheoretical calculations of solvation 12-Crown-4 (12CN4) in aqueous solution and its experimental interaction with nano CuSO4
Theoretical study of the electronic structure, and nonlinear optical properties (NLO) analysis of 12-crown-4were done using Density Functional Theory (DFT) evaluations at the B3LYP/6-311G (d,p) level of theory. The optimized structure is nonlinear compound as indicated from the dihedral angles were presented. The calculated EHOMO and ELUMO energies of 12-Crown-4 (12CN4) ca...
متن کاملTheoretical calculations of solvation 12-Crown-4 (12CN4) in aqueous solution and its experimental interaction with nano CuSO4
Theoretical study of the electronic structure, and nonlinear optical properties (NLO) analysis of 12-crown-4were done using Density Functional Theory (DFT) evaluations at the B3LYP/6-311G (d,p) level of theory. The optimized structure is nonlinear compound as indicated from the dihedral angles were presented. The calculated EHOMO and ELUMO energies of 12-Crown-4 (12CN4) ca...
متن کاملTheoretical Study of 1,4-Dioxane in Aqueous Solution and Its Experimental Interaction with Nano-CuSO4
The electronic structure, Non-Linear Optical (NLO) properties and Natural Bonding Orbital (NBO) analysis of 1,4-dioxane were investigated using the theoretical study of Density Functional Theory (DFT) calculations at the B3LYP/6-311G (d,p) level of theory. The optimized structure is nonlinear as indicated from the dihedral angles. Natural bonding orbital analysis has been analyzed in terms...
متن کاملSearch for short-time phase effects in the electronic damage evolution - a case study with silicon
This work focusses on the production and decay properties of inner-shell vacancies and valence-band excitations induced by swift highly charged ions interacting with amorphous and crystalline Si. High resolution electron spectra have been taken for fast heavy ions at 1.78 to 5 MeV/u as well as for electrons of similar velocity incident on atomically clean Si targets of well defined phase. Vario...
متن کامل